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But I'm wondering lately, does the sound quality of these emulated sound format have a real difference with the original OST (the SPC, GYM, PSF, PSF2)?
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In the ideal case (OST being recorded directly from the game without changes, sound format emulated perfectly) there should no difference at all (and perfectly emulated native emulate formats are superior to lossy formats like MP3).
I honestly don't understand why one would want to compare both though, by far the most game music is not available as OSTs, one calling proven emulated sound formats imperfect would lead to missing out a lot of music.
Emulated sound formats of newer systems have the advantage that you can tweak the sound, e.g. you can disable reverb used in SNES/PS1/PS2 scores to hear the actual score more clearly.
Jam it back in, in the dark.