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Toshihiko Sahashi : The BigO,Kateikyoushi Hitman Reborn.
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Obligatory mention of Gunslinger Girl because that's still my favorite anime OST of all time as well as a series on my top 10 list for having such a great emotional story that has a good mix of action in it.
I'd also suggest taking a look at Red Garden. While some of the vocals in the series might sound a bit jarring and poorly executed, the rest of the soundtrack is actually really good and it may very well be the best soundtrack (rivaled by Clannad perhaps) from an anime that was shown in 2007. It also helps that the plot and character development are both awesome and that it's the best Gonzo show to have come out since Gankutsuou. Better than Bokurano even.
Jam it back in, in the dark.
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