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Same for ActRaiser music but props for Terminus for having played Legaia: Dual Saga, I didn't think anyone else had played that game.
Phantasy Star III:
I loved Phantasy Star III's gloomy music and its battle music the most. What made it stand out quite a bit was the battle music would change according the level of difficulty you'll enter the battle with. This IS awesome, and refreshing and entirely new to me at the time that I appreciated every bit of those tracks.
And not only that music differs, when you're in the overworld, depending on if you're traveling solo or however many in a party, that music changes too (4 in all).
Of course right away... solo ground trek music here.